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EXPERIMENTAL AND NUMERICAL ANALYSIS OF SAWDUST-CHAR COMBUSTION REACTIVITY IN A DROP TUBE REACTOR

机译:滴管反应器中木屑-焦炭燃烧反应性的实验和数值分析

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摘要

This article discusses the results of a combined experimental and numerical investigation of the combustion reactivity of sawdust char in a drop tube furnace. The work presented here was motivated by the lack of reliable data in the open literature on the combustion reactivity of woody biomass char. This study involved the experimental determination of the global kinetic param- eters of sawdust-char oxidation and the subsequent application of these parameters in a computational fluid dynamics (CFD) code. The modified code was employed for mathematical modeling of the sawdust-char combustion in the drop tube furnace. The experiments were conducted at furnace tempera- tures of 1473 and 1673 K in a 10mol% O_2 environment and 1473 K in air. Experimental results indicated that the bulk of the char oxidation reaction for sawdust occurred in Regime II where chemical reaction and pore diffusion rates are comparable. In addition, the sawdust char exhibited distinctive near- extinction combustion behavior at the early stage of the reaction. The com- bustion reactivity of the sawdust char, with an apparent reaction order (n) of 0.4, was comparable to that of some high-volatile bituminous coal chars. Good agreement was achieved between predicted and experimental results.
机译:本文讨论了在滴管式炉中对木屑炭的燃烧反应性进行综合实验和数值研究的结果。本文介绍的工作是由于缺乏有关木质生物质焦炭燃烧反应性的公开文献的可靠数据而激发的。这项研究涉及对木屑炭氧化总体动力学参数的实验确定,以及随后在计算流体力学(CFD)代码中应用这些参数。修改后的代码用于滴管式炉中锯末炭燃烧的数学建模。实验是在10%的O_2环境中在1473和1673 K的炉温下以及在空气中在1473 K的炉温下进行的。实验结果表明,木屑的焦炭氧化反应大部分发生在制度II中,化学反应和孔扩散速率可比。另外,在反应的早期,木屑炭表现出独特的近乎熄灭的燃烧行为。锯末焦的燃烧反应性(n)为0.4,可与某些高挥发性烟煤焦相比。预测结果与实验结果之间取得了良好的一致性。

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