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Effect of typhoon on atmospheric aerosol particle pollutants accumulation over Xiamen, China

机译:台风对厦门市大气气溶胶颗粒污染物累积的影响

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摘要

Great influence of typhoon on air quality has been confirmed, however, rare data especially high time resolved aerosol particle data could be used to establish the behavior of typhoon on air pollution. A single particle aerosol spectrometer (SPAMS) was employed to characterize the particles with particle number count in high time resolution for two typhoons of Soulik (2013) and Soudelor (2015) with similar tracks. Three periods with five events were classified during the whole observation time, including pre - typhoon (event 1 and event 2), typhoon (event 3 and event 4) and post - typhoon (event 5) based on the meteorological parameters and particle pollutant properties. First pollutant group appeared during pre typhoon (event 2) with high relative contributions of V - Ni rich particles. Pollution from the ship emissions and accumulated by local processes with stagnant meteorological atmosphere dominated the formation of the pollutant group before typhoon. The second pollutant group was present during typhoon (event 3), while typhoon began to change the local wind direction and increase wind speed. Particle number count reached up to the maximum value. High relative contributions of V - Ni rich and dust particles with low value of NO3-/SO42- was observed during this period, indicating that the pollutant group was governed by the combined effect of local pollutant emissions and long-term transports. The analysis of this study sheds a deep insight into understand the relationship between the air pollution and typhoon. (C) 2016 Elsevier Ltd. All rights reserved.
机译:台风对空气质量的影响已经得到确认,但是,稀有数据,尤其是高分辨的气溶胶颗粒数据,可以用来确定台风对空气污染的行为。使用单颗粒气溶胶光谱仪(SPAMS)来表征具有类似轨迹的两个Soulik(2013)和Soudelor(2015)台风的高分辨分辨率的颗粒数计数的颗粒。根据气象参数和颗粒污染物的性质,在整个观测时间内将三个时段分为五个事件,包括台风前(事件1和事件2),台风(事件3和事件4)和台风后(事件5)。 。在台风发生前(事件2),第一个污染物组出现了,其中富含V-Ni相对颗粒。在台风之前,船舶排放的污染物以及气象过程停滞的局部过程累积的污染物占主导地位。第二类污染物是在台风期间出现的(事件3),而台风开始改变当地的风向并增加风速。颗粒数达到最大值。在此期间,观察到较高的V-富镍和尘埃颗粒(NO3- / SO42-值较低)的相对贡献,表明污染物组受当地污染物排放和长期运输的共同影响。这项研究的分析为深入了解空气污染与台风之间的关系提供了深刻的见识。 (C)2016 Elsevier Ltd.保留所有权利。

著录项

  • 来源
    《Chemosphere》 |2016年第9期|244-255|共12页
  • 作者单位

    SOA, Key Lab Global Change & Marine Atmospher Chem, Inst Oceanog 3, Xiamen 361005, Peoples R China;

    SOA, Key Lab Global Change & Marine Atmospher Chem, Inst Oceanog 3, Xiamen 361005, Peoples R China;

    SOA, Key Lab Global Change & Marine Atmospher Chem, Inst Oceanog 3, Xiamen 361005, Peoples R China;

    SOA, Key Lab Global Change & Marine Atmospher Chem, Inst Oceanog 3, Xiamen 361005, Peoples R China;

    SOA, Key Lab Global Change & Marine Atmospher Chem, Inst Oceanog 3, Xiamen 361005, Peoples R China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Aerosol particles; Size distribution; Chemical composition; Pollutant accumulation; Typhoon;

    机译:气溶胶颗粒;粒度分布;化学成分;污染物积累;台风;

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