An unexpected role of the monodentate ligand in photocatalytic hydrogen production of the pentadentate ligand-based cobalt complexes

Jingfan Xie; Qianxiong Zhou; Chao Li; Weibo Wang; Yuanjun Hou; Baowen Zhang; Xuesong Wang

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An unexpected role of the monodentate ligand in photocatalytic hydrogen production of the pentadentate ligand-based cobalt complexes

机译：单齿配体在基于五齿配体的钴配合物的光催化制氢中的出乎意料的作用

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摘要

The dissociation of one pyridine of a pentadentate ligand (N4Py) from the Co centre was found to be responsible for the formation of a Co(Ⅲ) hydride species, an indispensable intermediate for photo- catalytic proton reduction.

机译：发现五齿配体（N4Py）的一个吡啶从Co中心解离是形成Co（Ⅲ）氢化物的原因，Co（Ⅲ）氢化物是光催化质子还原必不可少的中间体。

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《Chemical Communications》 |2014年第49期|6520-6522|共3页
作者
Jingfan Xie; Qianxiong Zhou; Chao Li; Weibo Wang; Yuanjun Hou; Baowen Zhang; Xuesong Wang;
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作者单位

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China,Graduate School of Chinese Academy of Sciences, Beijing 100049, P. R. China;

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;

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1. Electro- and Photocatalytic Hydrogen Production by Molecular Cobalt Complexes With Pentadentate Ligands [J] . Zhao Xuan, Wang Ping, Long Melissa Comments on Inorganic Chemistry: A Journal of Critical Discussion of the Current Literature . 2017,第1a6期

机译：用五边形配体的分子钴配合物电和光催化氢气产生
2. ELECTRO- AND PHOTOLYTIC HYDROGEN PRODUCTION BY MONONUCLEAR COBALT COMPLEXES WITH PENTADENTATE LIGANDS [J] . Xuan Zhao, Michael Yanney, Manohar Vennampalli, American Chemical Society, Division of Fuel Chemistry, Preprints . 2015,第2cd期

机译：单齿钴配位化合物单核钴配合物生产电和光解氢
3. Isomeric distribution and catalyzed isomerization of cobalt(III) complexes with pentadentate macrocyclic ligands. Importance of hydrogen bonding [J] . Aullon G, Bernhardt PV, Bozoglian F, Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics . 2006,第21期

机译：具有五齿大环配体的钴（III）配合物的异构分布和催化异构化。氢键的重要性
4. ELECTRO- AND PHOTOLYTIC HYDROGEN PRODUCTION BY MONONUCLEAR COBALT COMPLEXES WITH PENTADENTATE LIGANDS [C] . Xuan Zhao, Michael Yanney, Manohar Vennampalli American Chemical Society National Meeting Exposition . 2015

机译：用五核钴配合物用五核配体的电气和光溶解氢气产生
5. MANGANESE(II) AND COBALT(III) COMPLEXES OF MULTIDENTATE LIGANDS: I. MANGANESE(II) COMPLEXES OF A MACROCYCLIC PENTADENTATE LIGAND. II. COBALT(III) COMPLEXES OF LINEAR TETRAMINE LIGANDS. [D] . HAMILTON, HOBART GORDON, JR. 1968

机译：多齿配体的锰（II）和钴（III）配合物：I.大环戊二烯配体的锰（II）配合物。二。线性叔丁胺配体的钴（III）配合物。
6. Facile hydrogen atom transfer to iron(iii) imido radical complexes supported by a dianionic pentadentate ligand [O] . Denis M. Spasyuk, Stephanie H. Carpenter, Christos E. Kefalidis, 2016

机译：氢原子容易转移到双齿五齿配体支持的亚铁亚铁自由基络合物中
7. Isomeric Distribution and Catalyzed Isomerization of Cobalt(III) Complexes with Pentadentate Macrocyclic Ligands. Importance of Hydrogen Bonding [O] . -1

机译：用五环丙烯酸盐配体的钴（III）配合物的异构分布和催化异构化。氢键的重要性
8. Manganese(II) and Manganese(III) Complexes of Linear Pentadentate Schiff Base Ligands [R] . Coleman, W. M. 1980

机译：线性五齿schiff碱配体的锰（II）和锰（III）配合物

An unexpected role of the monodentate ligand in photocatalytic hydrogen production of the pentadentate ligand-based cobalt complexes

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