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1D/2D heterostructure nanofiber flexible sensing device with efficient gas detectivity

机译:具有高效气体检测能力的一维/二维异质结构纳米纤维柔性传感装置

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摘要

Wearable and flexible chemical sensors are attracting attention for the healthcare and environmental applications due to their desirable operation safety, high flexible and enable to realize real-time detection. However, a major challenge in creating flexible chemical sensors is the insufficient activity and durability of the materials currently employed as sensing layers for gas molecule adsorption and reaction. Herein, we describe an ultra-sensitive flexible sensing platform that was based on efficient 1D/2D hetero-structure nanofiber consisting of a 1D TiO2 nanofiber wrapped in a shell of Bi2WO6 nanosheets. We also demonstrated the well-designed multi-channel sensitization effects in the electrosensitive, including the unique structural advantage, the grain boundary effect, and hetero-interface effect could synergistically improve electronic transform and gas molecules absorption at the interfaces. As a result, flexible sensor based on the 1D/2D hetero-structure nanofiber exhibit good mechanical stable and high selective sensitivity to ethanol gas molecules under room temperature. Thus, the introduction of hetero-interface and grain boundary provides a new avenue towards realizing highly sensitive and stable flexible sensing device.
机译:穿戴式和柔性化学传感器以其理想的操作安全性,高度的柔性并能够实现实时检测而吸引了医疗保健和环境应用的关注。然而,创建柔性化学传感器的主要挑战是目前用作气体分子吸附和反应传感层的材料的活性和耐久性不足。在这里,我们描述了一种超灵敏的柔性传感平台,该平台基于高效的1D / 2D异质结构纳米纤维,该纤维由包裹在Bi2WO6纳米片壳中的1D TiO2纳米纤维组成。我们还展示了电敏性中精心设计的多通道敏化效应,包括独特的结构优势,晶界效应和异质界面效应可以协同改善界面处的电子转化和气体分子吸收。结果,基于1D / 2D异质结构纳米纤维的柔性传感器在室温下表现出良好的机械稳定性和对乙醇气体分子的高选择性敏感性。因此,异质界面和晶界的引入为实现高度灵敏,稳定的柔性传感装置提供了新途径。

著录项

  • 来源
    《Applied Surface Science》 |2019年第15期|209-215|共7页
  • 作者单位

    Jilin Univ, Coll Elect Sci & Engn, State Key Lab Integrated Optoelect, Changchun 130012, Jilin, Peoples R China;

    Jilin Univ, Inst Theoret Chem, Lab Theoret & Computat Chem, Changchun 130012, Jilin, Peoples R China;

    Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China|Chinese Acad Sci, Inst Elect, State Key Lab Transducer Technol, Beijing 100190, Peoples R China;

    Shenzhen Technol Univ, Coll Hlth & Environm Engn, Shenzhen 518118, Peoples R China;

    Jilin Univ, Coll Elect Sci & Engn, State Key Lab Integrated Optoelect, Changchun 130012, Jilin, Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Flexible sensing device; 1D/2D hetero-nanofiber; Grain boundary; Hetero-interface; High sensing properties; Mechanical stable;

    机译:柔性传感装置;一维/二维异质纤维;晶界;异质界面;高传感性能;机械稳定;

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