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Reduced graphene oxide supported Au nanoparticles as an efficient catalyst for aerobic oxidation of benzyl alcohol

机译:还原的氧化石墨烯负载的金纳米颗粒作为有氧氧化苯甲醇的有效催化剂

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摘要

Various Au/C catalysts were prepared by Au nanoparticels supported on different carbonaceous supports including reduced graphene oxide (RGO), activated carbon (AC) and graphite (GC) using sol-immobilization method. Au/RGO shows a much higher activity than Au/AC and Au/GC in the liquid phase aerobic oxidation of benzyl alcohol. The superior catalytic performance of Au/RGO may be related to the presence of surface O-containing functional groups and moderate graphite character of RGO supports.
机译:利用溶胶固定法,通过负载在不同碳质载体上的金纳米颗粒制备了各种金/碳催化剂,所述碳质载体包括还原性氧化石墨烯(RGO),活性炭(AC)和石墨(GC)。在苯甲醇的液相好氧氧化中,Au / RGO显示出比Au / AC和Au / GC高得多的活性。 Au / RGO的优异催化性能可能与表面含O官能团的存在和RGO载体的适度石墨特性有关。

著录项

  • 来源
    《Applied Surface Science》 |2013年第1期|450-455|共6页
  • 作者单位

    Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, China;

    Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, China;

    Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, China;

    Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, China,CAS Key Laboratory of Materials for Energy Conversion, University of Science and Technology of China, Hefei 230026, China,Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, China;

    Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, China;

    Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, China,CAS Key Laboratory of Materials for Energy Conversion, University of Science and Technology of China, Hefei 230026, China,Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Gold; Reduced graphene oxide; Alcohol oxidation; TPD; Raman;

    机译:金;氧化石墨烯还原;酒精氧化;TPD;拉曼;

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