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Zn-3(OH)(2)V2O7 center dot 2H(2)O/g-C3N4: A novel composite for efficient photodegradation of methylene blue under visible-light irradiation

机译:Zn-3(OH)(2)V2O7中心点2H(2)O / g-C3N4:一种新型复合材料,可在可见光照射下有效地光降解亚甲基蓝

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摘要

In this work, we used a facile method to prepare a series of Zn-3(OH)(2)V2O7 center dot 2H(2)O/g-C3N4 composites in a 70 degrees C water bath for 10 h and characterized them by X-ray diffraction (XRD), scanning electron microscopy (SEM), UV-vis diffuse reflectance spectroscopy (DRS), Brunauer-Emmett-Teller (BET), and photoluminescence (PL). Degradation of methylene blue (MB) and phenol were carried out to evaluate the photocatalytic activities of samples under visible light irradiation. Presence of Zn-3(OH)(2)V2O7 center dot 2H(2)O increased surface areas and promoted the charge separation, exerted great influence on the photocatalytic activity and absorption capacity of g-C3N4. In addition, the synergic effect was explained and a possible photocatalytic mechanism was proposed. (C) 2015 Elsevier B.V. All rights reserved.
机译:在这项工作中,我们使用一种简便的方法在70摄氏度的水浴中制备了一系列Zn-3(OH)(2)V2O7中心点2H(2)O / g-C3N4复合材料,并对它们进行了表征X射线衍射(XRD),扫描电子显微镜(SEM),紫外可见漫反射光谱(DRS),Brunauer-Emmett-Teller(BET)和光致发光(PL)。进行了亚甲基蓝(MB)和苯酚的降解,以评估样品在可见光照射下的光催化活性。 Zn-3(OH)(2)V2O7中心点2H(2)O的存在增加了表面积并促进了电荷分离,对g-C3N4的光催化活性和吸收能力产生了很大影响。此外,解释了协同作用并提出了可能的光催化机理。 (C)2015 Elsevier B.V.保留所有权利。

著录项

  • 来源
    《Applied Surface Science》 |2015年第30期|602-609|共8页
  • 作者单位

    Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Peoples R China;

    Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Peoples R China;

    Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Peoples R China;

    Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Peoples R China;

    Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Peoples R China;

    Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Peoples R China;

    S China Univ Technol, Coll Mat Sci & Engn, Guangzhou 510640, Guangdong, Peoples R China;

    Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Zn-3(OH)(2)V2O7 center dot 2H(2) O/g-C-3 N-4; Composites; Photodegradation; Synergic effect; Visible light;

    机译:Zn-3(OH)(2)V2O7中心点2H(2)O / g-C-3 N-4;复合材料;光降解;协同效应;可见光;

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