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Fabrication of conductive and high-dispersed Ppy@Ag/g-C3N4 composite photocatalysts for removing various pollutants in water

机译:导电型高分散Ppy @ Ag / g-C3N4复合光催化剂的制备用于去除水中各种污染物

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The ternary conductive Ppy@Ag/g-C3N4 composite photocatalysts was successfully synthesized by polymerization process and surface polymerization technique. And the as-prepared Ppy@Ag/g-C3N4 sample exhibited the higher photocatalytic activity for various pollutant (MO, DM, TC, CIP, GFLX and EH) remove than that of pure g-C3N4 and Ag/g-C3N4 under visible light irradiation. It mainly originated from the Ag nanoparticles anchored between g-C3N4 and Ppy acted as electron transfer mediator that facilitated the charge carrier separation and then expending the lifetime of the carriers. Meanwhile, the obtained Ppy@Ag/g-C3N4 sample also showed a relatively good recycling stability which was the crucial factor for photocatalyst practical application. This work provided a new facile strategy for improving photo-degradation activity of g-C3N4 photocatalyst. (C) 2016 Elsevier B.V. All rights reserved.
机译:通过聚合工艺和表面聚合技术成功地合成了三元导电Ppy @ Ag / g-C3N4复合光催化剂。制备的Ppy @ Ag / g-C3N4样品在可见光下对各种污染物(MO,DM,TC,CIP,GFLX和EH)的去除表现出比纯g-C3N4和Ag / g-C3N4更高的光催化活性。光照射。它主要源自锚定在g-C3N4和Ppy之间的Ag纳米粒子,充当电子转移介质,促进电荷载流子分离,进而延长载流子的寿命。同时,所得的Ppy @ Ag / g-C3N4样品还显示出相对较好的循环稳定性,这是光催化剂实际应用的关键因素。这项工作为提高g-C3N4光催化剂的光降解活性提供了一种新的简便策略。 (C)2016 Elsevier B.V.保留所有权利。

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