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A Bioinspired Elastic Hydrogel for Solar-Driven Water Purification

机译:用于太阳能驱动的水净化的生物悬浮弹性水凝胶

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摘要

The global demand for clean and safe water will continue to grow well into the 21st century. Moving forward, the lack of access to clean water, which threatens human health and strains precious energy resources, will worsen as the climate changes. Therefore, future innovations that produce potable water from contaminated sources must be sustainable. Inspired by nature, a solar absorber gel (SAG) is developed to purify water from contaminated sources using only natural sunlight. The SAG is composed of an elastic thermoresponsive poly(N-isopropylacrylamide) (PNIPAm) hydrogel, a photothermal polydopamine (PDA) layer, and a sodium alginate (SA) network. Production of the SAG is facile; all processing is aqueous-based and occurs at room temperature. Remarkably, the SAG can purify water from various harmful reservoirs containing small molecules, oils, metals, and pathogens, using only sunlight. The SAG relies on solar energy to drive a hydrophilic/hydrophobic phase transformation at the lower critical solution temperature. Since the purification mechanism does not require water evaporation, an energy-intensive process, the passive solar water-purification rate is the highest reported. This discovery can be transformative in the sustainable production of clean water to improve the quality of human life.
机译:全球对清洁和安全的水需求将继续进入21世纪。向前发展,缺乏威胁人类健康和诱饵能源资源的清洁水的进入将会随着气候变化而恶化。因此,未来创新从污染的来源生产饮用水必须是可持续的。灵感来自大自然,开发了一种太阳能吸收凝胶(SAG),仅使用自然阳光从污染的来源净化水。 SAG由弹性热反应性聚(N-异丙基丙烯酰胺)(PNIPAM)水凝胶,光热聚亚多胺(PDA)层和藻酸钠(SA)网络组成。落下的生产是宽容的;所有加工都是基于含水的,在室温下发生。值得注意的是,使用仅使用阳光,张力可以从包含小分子,油,金属和病原体的各种有害储层净化水。下垂依赖于太阳能在临界溶液温度下驱动亲水/疏水相变。由于净化机制不需要水蒸发,所以能量密集的过程,被动太阳能水净化率是最高报道的。这一发现可以在洁净水的可持续生产中转化,以提高人类生活的质量。

著录项

  • 来源
    《Advanced Materials》 |2021年第18期|2007833.1-2007833.9|共9页
  • 作者单位

    Princeton Univ Dept Chem & Biol Engn Princeton NJ 08544 USA;

    Princeton Univ Dept Chem & Biol Engn Princeton NJ 08544 USA|Princeton Univ Princeton Inst Sci & Technol Mat Princeton NJ 08544 USA;

    Princeton Univ Dept Chem & Biol Engn Princeton NJ 08544 USA|Princeton Univ Princeton Inst Sci & Technol Mat Princeton NJ 08544 USA;

    Princeton Univ Princeton Inst Sci & Technol Mat Princeton NJ 08544 USA|Princeton Univ Dept Mech & Aerosp Engn Princeton NJ 08544 USA;

    Princeton Univ Dept Chem & Biol Engn Princeton NJ 08544 USA;

    Princeton Univ Dept Chem & Biol Engn Princeton NJ 08544 USA|Princeton Univ Princeton Inst Sci & Technol Mat Princeton NJ 08544 USA;

  • 收录信息
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    clean water production; gels; poly(N#8208; isopropyl acrylamide); polydopamine; solar absorption;

    机译:清洁水生产;凝胶;聚(N‐异丙基丙烯酰胺);多茶胺;太阳能吸收;

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