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Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks

机译:评估静态长度尺度在多分散硬盘中玻璃动力学背后的作用

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摘要

The possible role of growing static order in the dynamical slowing down toward the glass transition has recently attracted considerable attention. On the basis of random first-order transition theory, a new method to measure the static correlation length of amorphous order, called “point-to-set” (PTS) length, has been proposed and used to show that the dynamic length grows much faster than the static length. Here, we study the nature of the PTS length, using a polydisperse hard-disk system, which is a model that is known to exhibit a growing hexatic order upon densification. We show that the PTS correlation length is decoupled from the steeper increase of the correlation length of hexatic order and dynamic heterogeneity, while closely mirroring the decay length of two-body density correlations. Our results thus provide a clear example that other forms of order can play an important role in the slowing down of the dynamics, casting a serious doubt on the order-agnostic nature of the PTS length and its relevance to slow dynamics, provided that a polydisperse hard-disk system is a typical glass former.
机译:最近,逐渐增加的静态顺序在向玻璃化转变的动态减速中的可能作用引起了相当大的关注。在随机一阶跃迁理论的基础上,提出了一种测量非晶态静态相关长度的新方法,称为“点对集”(PTS)长度,用于表明动态长度会大大增加。比静态长度快。在这里,我们使用多分散硬盘系统研究了PTS长度的性质,该系统是一种已知在致密化过程中显示出不断增长的六价序的模型。我们显示,PTS相关长度与六次有序相关长度和动态异质性的急剧增加解耦,同时紧密反映了两体密度相关的衰减长度。因此,我们的结果提供了一个明确的例子,即其他形式的订单在减慢动力学过程中可能起重要作用,这对PTS长度的不可知顺序性质及其与慢速动力学的相关性提出了严重怀疑,前提是多分散性硬盘系统是典型的玻璃成型机。

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