Induced Rayleigh and Hyper-Rayleigh Spectra Pair Hyperpolarizability

摘要

Collision-induced (CI) Rayleigh and hyper-Rayleigh (HR) light scattering spectra are briefly discussed. The CI hyperpolarizability for D_(∞h) molecule-atom system is studied. Results are applied to the case of H_2-Ar pair. Spherical components △β_(01)~(s.1)(R) △β_(21)~(s,1)(R),△β_(23)~(s,1)(R) and △β_(45)~(s,1)(R) of the dipole part of the H_2-Ar first hyperpolarizability tensor △β~→ are computed.