Direct Probing of the Local Solvent ResponseDuring Intermolecular Electron Transfer

摘要

Following resonant photo-excitation of coumarin 152 in the electron donatingrnsolvents aniline and dimethylaniline, dramatic changes the local intermolecular solvent responsernare monitored directly as a function of time during intermolecular electron transferrnusing third-order non-resonant Raman spectroscopy.