Electrolytes for Rechargeable Lithium–Air Batteries

Lai Jingning; Xing Yi; Chen Nan; Li Li; Wu Feng; Chen Renjie

摘要

Abstract >Lithium–air batteries are promising devices for electrochemical energy storage because of their ultrahigh energy density. However, it is still challenging to achieve practical Li–air batteries because of their severe capacity fading and poor rate capability. Electrolytes are the prime suspects for cell failure. In this Review, we focus on the opportunities and challenges of electrolytes for rechargeable Li–air batteries. A detailed summary of the reaction mechanisms, internal compositions, instability factors, selection criteria, and design ideas of the considered electrolytes is provided to obtain appropriate strategies to meet the battery requirements. In particular, ionic liquid (IL) electrolytes and solid‐state electrolytes show exciting opportunities to control both the high energy density and safety. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P>锂 - 空气电池是电化学能量储存的有希望的设备，因为它们的超高能量密度。然而，由于其严重的容量衰落和差价能力，实现实用的LI-Air电池仍然具有挑战性。电解质是细胞衰竭的主要嫌疑人。在这篇综述中，我们专注于可充电Li-Air电池的电解质的机遇和挑战。提供了反应机制，内部组合物，不稳定因子，选择标准和设计考虑的详细概述，以获得适当的策略以满足电池要求。特别地，离子液体（IL）电解质和固态电解质显示出令人兴奋的机会，以控制高能量密度和安全性。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第8期</span><b style="margin: 0 2px;">|</b><span>共24页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lai Jingning&option=202" target="_blank" rel="nofollow">Lai Jingning;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xing Yi&option=202" target="_blank" rel="nofollow">Xing Yi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Nan&option=202" target="_blank" rel="nofollow">Chen Nan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Li&option=202" target="_blank" rel="nofollow">Li Li;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Feng&option=202" target="_blank" rel="nofollow">Wu Feng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Renjie&option=202" target="_blank" rel="nofollow">Chen Renjie;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Beijing Key Laboratory of Environmental Science and EngineeringBeijing Institute of TechnologyBeijing 100081 China;</p> <p>Beijing Key Laboratory of Environmental Science and EngineeringBeijing Institute of TechnologyBeijing 100081 China;</p> <p>Beijing Key Laboratory of Environmental Science and EngineeringBeijing Institute of TechnologyBeijing 100081 China;</p> <p>Beijing Key Laboratory of Environmental Science and EngineeringBeijing Institute of TechnologyBeijing 100081 China;</p> <p>Beijing Key Laboratory of Environmental Science and EngineeringBeijing Institute of TechnologyBeijing 100081 China;</p> <p>Beijing Key Laboratory of Environmental Science and EngineeringBeijing Institute of TechnologyBeijing 100081 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=aprotic electrolytes&option=203" rel="nofollow">aprotic electrolytes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=aqueous electrolytes&option=203" rel="nofollow">aqueous electrolytes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ionic-liquid electrolytes&option=203" rel="nofollow">ionic-liquid electrolytes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium–air batteries&option=203" rel="nofollow">lithium–air batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=solid-state electrolytes&option=203" rel="nofollow">solid-state electrolytes;</a> </p> <div class="translation"> 机译：非质子电解质;水性电解质;离子液体电解质;锂气体;固态电解质; 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2021-07-30</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130408709376.html">ELECTROLYTE ADDITIVES FOR RECHARGEABLE LITHIUM BATTERY ELECTROLYTE FOR RECHARGEABLE LITHIUM BATTERY AND RECHARGEABLE LITHIUM BATTERY INCLUDING THE SAME</a> <b>[P]</b> . <span> 外国专利：  KR20170058707A </span> <span> . 2017-05-29</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于可充电锂电池的电解液添加剂用于可充电锂电池的电解液和可充电锂电池，包括相同的电解液 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130414222227.html">ELECTROLYTE FOR LITHIUM AIR RECHARGEABLE BATTERY AND LITHIUM AIR RECHARGEABLE BATTERY INCLUDING THE SAME</a> <b>[P]</b> . <span> 外国专利：  KR20150051316A </span> <span> . 2015-05-12</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：锂空气可充电电池的电解液和锂空气可充电电池（包括相同的电解液） </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130414257977.html">ELECTROLYTE FOR LITHIUM AIR RECHARGEABLE BATTERY AND LITHIUM AIR RECHARGEABLE BATTERY INCLUDING THE SAME</a> <b>[P]</b> . <span> 外国专利：  KR20150015643A </span> <span> . 2015-02-11</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：锂空气可充电电池的电解液和锂空气可充电电池（包括相同的电解液） </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 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