Spatial and temporal distribution of methane emissions from a covered landfill equipped with a gas recollection system

摘要

A previously developed surface probe method, which allows for instantaneous methane (CH_4) flux measurement, was used to establish CH_4 emission maps of a municipal landfill with a final clay cover and equipped with a gas recollection system. In addition to spatial variations, the method was applied at 7 different times over a total timeframe of 65 h and under similar weather conditions to determine the intrinsic temporal variations of CH_4 emissions; i.e., the temporal variation related to the dynamic of the landfill rather than the one driven by external factors. Furthermore, continuous CH_4 fluxes, with a data acquisition frequency of 1 Hz, were measured during 12 h at a single position, and for one hour at 22 locations of the landfill, spanning a large range of CH_4 emission magnitudes. A simple model for the numerical characterization of spatiotemporal variability of the landfill emission was used and allowed us to separately quantify the temporal and spatial variability. This model showed that, in the landfill tested, the temporal distribution of CH_4 emissions resulted more homogeneous than the spatial distribution. Other attributes of the temporal and spatial distributions of CH_4 emissions were also established including the anisotropic nature of the spatial distribution and, contrastingly, the stochastic temporal variability of such emissions.