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Integration of a rapid scanning technique into THz time-domain spectrometers for nonlinear THz spectroscopy measurements

机译:将快速扫描技术集成到THz时域光谱仪中以进行非线性THz光谱测量

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摘要

We have implemented a rapid scanning technique into THz time-domain spectrometers using an oscillating frictionless delay line, especially adapted for nonlinear THz experiments. Thereby we were able to increase the dynamic range of THz measurements in the frequency range from 40 to 200 cm-1 by up to 24 dB and reduce the scanning time by up to a factor of 200. We report here test measurements on TDS-setups at repetition rates of 80 MHz and 5 kHz. The dynamic range exceeds 64 dB, which allows to record even small changes in the THz absorption upon optical excitation by a THz probe, covering the frequency range of the intermolecular modes and the phonon bands. We demonstrate the potential of this technique for optical-pump THz-probe experiments using a 70 μm thick high-resistivity silicon, excited by 400 nm, ∼50 fs pulses as a sample.
机译:我们已经使用振荡无摩擦延迟线在THz时域光谱仪中实施了快速扫描技术,特别适用于非线性THz实验。因此,我们能够在40到200 cm -1 的频率范围内将THz测量的动态范围增加多达24 dB,并将扫描时间减少了多达200倍。此处以80 MHz和5 kHz的重复频率测试TDS设置的测量结果。动态范围超过64 dB,这允许在THz探头进行光激发时记录THz吸收的很小变化,覆盖了分子间模式和声子带的频率范围。我们证明了该技术在光泵THz探针实验中的潜力,该实验使用厚度为70μm的高电阻率硅,被400 nm激发的〜50 fs脉冲作为样本。

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